Life Cycle Assessment of DMC Produced with the Commercial “Eni” Process

Timeline


March 2024 - June 2024


Client

Northwestern University

Problem Statement

Conventional production of dimethyl carbonate (DMC) relies heavily on fossil fuels and generates significant environmental impact. As DMC demand grows with electrification, sustainable alternatives are urgently needed.

This project explored the feasibility of producing DMC via an electrochemical process powered by renewable electricity. Using life cycle assessment (LCA), the team evaluated environmental trade-offs, cost drivers, and system design to compare this green method against conventional approaches.

Project Overview and Scope

Goal : Evaluate electrochemical production of DMC as a sustainable alternative to fossil-based methods.

1. Process Design : Modeled electrochemical DMC production using CO₂ and methanol. Process flow diagram built in Aspen Plus with reactor, separation, and recovery steps.
2. LCA : Created life cycle inventory using ecoinvent, GREET and literature data. Used TRACI 2.1 for impact categories (e.g., GHG emissions, acidification, fossil depletion).
3. Scenario & Sensitivity Analysis : Tested impacts of electricity source (wind, solar, grid). Analyzed sensitivity to efficiency, recovery, and separation performance.
4. Technoeconomic Analysis: Estimated capital & operating costs. Compared levelized cost across scenarios.

LCA results for the electrochemical process for DMC production by unit operation and electricity source.

Tools and Applications Used

Aspen HYSYS- used for process modelling and energy requirements
GREET - Used to estimate emissions profiles and fuel cycle energy use
Ecoinvent - Used as the basis for comparing both electrochemical and conventional production routes
Microsoft Excel- for graphing and data collection
 

Project Documents

Click here to see our full report

Click here to see our presentation